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Abstract Two papers recently reported the detection of gaseous nickel and iron in the comae of over 20 comets from observations collected over two decades, including interstellar comet 2I/Borisov. To evaluate the state of the laboratory data in support of these identifications, we reanalyzed archived spectra of comet C/1996 B2 (Hyakutake), one of the nearest and brightest comets of the past century, using a combined experimental and computational approach. We developed a new, many-level fluorescence model that indicates that the fluorescence emissions of Fe I and Ni I vary greatly with heliocentric velocity. Combining this model with laboratory spectra of an Fe-Ni plasma, we identified 22 lines of Fe I and 14 lines of Ni I in the spectrum of Hyakutake. Using Haser models, we estimate the nickel and iron production rates as Q Ni = (2.6–4.1) × 10 22 s −1 and Q Fe = (0.4–2.8) × 10 23 s −1 . From derived column densities, the Ni/Fe abundance ratio log 10 [Ni/Fe] = −0.15 ± 0.07 deviates significantly from solar abundance ratios, and it is consistent with the ratios observed in solar system comets. Possible production and emission mechanisms are analyzed in the context of existing laboratory measurements. Based on the observed spatial distributions, excellent fluorescence model agreement, and Ni/Fe ratio, our findings support an origin consisting of a short-lived unknown parent followed by fluorescence emission. Our models suggest that the strong heliocentric velocity dependence of the fluorescence efficiencies can provide a meaningful test of the physical process responsible for the Fe I and Ni I emission. 

The recent detection of a neutron star merger by the LIGO collaboration has renewed interest in laboratory studies of r-process elements. Accurate modeling and interpretation of the electromagnetic transients following the mergers requires computationally expensive calculations of both the structure and opacity of all trans-iron elements. To date, the necessary atomic data to benchmark structure codes are incomplete or, in some cases, absent entirely. Within the available laboratory studies, the literature on Au I and Au II provides incomplete reports of the emission lines and level structures. We present a new study of Au I and Au II lines and levels by exposing a solid gold target to plasma in the Compact Toroidal Hybrid (CTH) experiment at Auburn University. A wavelength range from 187 to 800 nm was studied. In Au I, 86 lines are observed, 43 of which are unreported in the literature, and the energies of 18 5d9 6s 6p levels and 16 of the 18 known 5d9 6s 6d levels are corroborated by a least-squares level energy optimization. In Au II, 76 emission lines are observed, and 51 of the lines are unreported in the literature. For both Au I and Au II, the new lines predominantly originate from the most energetic of the known levels, and over half of the new Au II lines have wavelengths longer than 300 nm. For the estimated electron parameters of CTH plasmas at the gold target (ne~10^12 cm−3, Te~10 eV), two-electron transitions are similar in intensity to LS-allowed one-electron transitions.